Oa. Starykh et al., ORIGIN OF SPIN GAP IN CAV4O9 - EFFECTS OF FRUSTRATION AND LATTICE-DISTORTIONS, Physical review letters, 77(12), 1996, pp. 2558-2561
Spin gap behavior of CaV4O9 is studied by including the effects of fru
strating magnetic interactions and lattice distortions. The spectrum o
f triplet excitations is calculated for a Heisenberg model on the 1/5-
depleted square lattice. In the spin gap phase, the location of the mi
nima of the spectrum in the Brillouin zone is found to depend nontrivi
ally on the exchange parameters. Experimental consequences of the temp
erature-dependent lattice distortion including its effect on the unifo
rm susceptibility and the spin gap are explored.