Ss. Harilal et al., TEMPORAL AND SPATIAL EVOLUTION OF CA IN LASER-INDUCED PLASMA FROM GRAPHITE TARGET, Journal of applied physics, 80(6), 1996, pp. 3561-3565
Laser ablation of graphite has been carried out using 1.06 mu m radiat
ion from a Q-switched Nd:YAG laser and the time of flight distribution
of molecular C-2 present in the resultant plasma is investigated in t
erms of distance from the target as well as laser fluences employing t
ime resolved spectroscopic technique. At low laser fluences the intens
ities of the emission lines from C-2 exhibit only single peak structur
e while beyond a threshold laser fluence, emission from C-2 shows a tw
in peak distribution in time. The occurrence of the faster velocity co
mponent at higher laser fluences is explained as due to species genera
ted from recombination processes while the delayed peak is attributed
to dissociation of higher carbon clusters resulting in the generation
of C-2 molecule. Analysis of measured data provides a fairly complete
picture of the evolution and dynamics of C-2 species in the laser indu
ced plasma from graphite. (C) 1996 American Institute of Physics.