T. Kinoshita et al., DOUBLY SHAPED D-2 EXCITATION-SPECTRA OF CS AND RB ATOMS IN SUPERFLUID-HELIUM DUE TO A QUADRUPOLE BUBBLE SURFACE OSCILLATION, Physical review. B, Condensed matter, 54(9), 1996, pp. 6600-6607
Our recent experiments show that the D-2 excitation spectra of Cs and
Rb atoms in superfluid helium have doubly shaped profiles. Such line s
hapes are beyond the description of a simplified spherical atomic bubb
le model which explains properly general features of optical spectra o
f neutral atoms in liquid helium. This paper gives a theoretical expla
nation of the doubly shaped profiles, with a model that the bubble str
ucture of surrounding helium is not spherical, but is deformed instant
aneously by a quadrupole oscillation. The calculated energy level of t
he P-3/2 State of the deformed atomic bubble is split into two branche
s, giving the D-2 excitation line shape consisting of two components w
ith different peak intensities and widths. The obtained line shape agr
ees qualitatively with the observed one, which enables us to confirm t
he importance of the dynamic Jahn-Teller effect due to a quadrupole os
cillation of the atomic bubble surface induced by zero-point fluctuati
ons.