We report a detailed study of the Hall effect in Sr2RuO4, the first la
yered perovskite superconductor which does not contain copper (T-c con
gruent to 1 K). The Hall coefficient (R(H)) was measured at temperatur
es between 20 mK and 300 K, and an unusual dependence of R(H) on the a
pplied magnetic field was observed. R(H) has a strong temperature depe
ndence below 25 K, but below 1 K it saturates at a value of -1.15x10(-
10) m(3)/C. The Fermi surface of Sr2RuO4 is known from quantum oscilla
tion measurements, and since it is nearly two dimensional, it is possi
ble to derive a simple expression for R(H) using methods developed by
Ong [Phys. Rev. B 43, 193 (1991)]. We show that if the mean free path,
l, is assumed to be isotropic at low temperatures, it is possible to
make an accurate quantitative calculation of R(H) on the basis of the
known Fermi surface parameters.