Thin films of solid He-3 are excellent examples of two-dimensional mag
netic systems. The first atomic layer is a paramagnet at coverages whe
re the second solid layer exhibits either ferromagnetic or antiferroma
gnetic behavior, depending on the coverage. Grafoil, an exfoliated pro
duct of Union Carbide, is generally used as the substrate. However, th
e atomically smooth crystalline platelets of Grafoil are typically 100
Angstrom in diameter, so a substrate with larger platelets would be u
seful for magnetization studies where domain size is important. Exfoli
ated ZYH graphite, with platelets in excess of 4000 Angstrom, is a goo
d substitute for Grafoil. Adsorption isotherms and STM images for ZYH
are discussed, and an experimental cell for magnetization measurements
is described briefly.