Fabrication technology at the nanometer scale to develop advanced devi
ces and low-dimensional structures requires atomic-scale control of th
in-film growth, selective-area growth, and ultra-fine photolithography
. To develop such atomic-scale control techniques, advanced characteri
zation at the atomic-scale is needed. We are now investigating surface
and interface structures and ways to control growth modes by surface
modification, and also trying to develop methods that allow realtime o
bservation of thin-film crystal growth by using various methods of adv
anced materials analysis that use synchrotron radiation. This report p
resents recent results obtained by these techniques for S/GaAs and SrF
2/S/GaAs, Sb/GaAs, and inAs/Se/GaAs, and also describes preliminary re
sults from realtime crystal growth observation.