We introduce and demonstrate a general wave packet method for laser is
otope separation. In this scheme, laser excited molecular (or atomic)
wave packets of differing isotopes become spatially separated in the c
ourse of their long-time free evolution. In order to overcome the quan
tum spreading of wave packets, we make use of the phenomenon of reviva
ls. We demonstrate experimentally, with mixed Br-79(2)/Br-81(2) isotop
es, that significant control over the isotope ratio can be achieved in
a single shot.