DYNAMICAL BEHAVIOR OF MICROEMULSION AND SPONGE PHASES IN THERMAL-EQUILIBRIUM

Citation
M. Hennes et G. Gompper, DYNAMICAL BEHAVIOR OF MICROEMULSION AND SPONGE PHASES IN THERMAL-EQUILIBRIUM, Physical review. E, Statistical physics, plasmas, fluids, and related interdisciplinary topics, 54(4), 1996, pp. 3811-3831
Citations number
71
Categorie Soggetti
Physycs, Mathematical","Phsycs, Fluid & Plasmas
ISSN journal
1063651X
Volume
54
Issue
4
Year of publication
1996
Part
B
Pages
3811 - 3831
Database
ISI
SICI code
1063-651X(1996)54:4<3811:DBOMAS>2.0.ZU;2-0
Abstract
The dynamical behavior of microemulsion and sponge phases is studied w ith a time-dependent Ginzburg-Landau model. The model has been shown p reviously to capture many of the essential static properties of these systems. Using a field-theoretic perturbation theory, we calculate the frequency-dependent (complex) viscosity eta(omega), sound velocity c( omega) and damping D(omega), and the scattering intensity S(k,t) in bu lk and film contrast. The viscosity is almost frequency independent fo r small omega, then drops sharply at a characteristic frequency omega , corresponding to a characteristic relaxation time tau similar to 1/o mega. The same relaxation rime is also found to dominate the sound ve locity and damping. The characteristic frequency has the scaling form omegasimilar to xi(-6)Omega(q xi), where xi is the correlation length and q is the inverse domain size of the microemulsion structure. The scattering intensity S(k,t) decays exponentially in time t for large t with an algebraic prefactor t(-alpha), both in bulk and in film contr ast. In the latter case, we find there are several regimes of the wave vector k with different exponents alpha.