Ct. Ying et al., SOLUTION OF THE DIFFUSION-EQUATIONS IN A GAS CENTRIFUGE FOR SEPARATION OF MULTICOMPONENT MIXTURES, Separation science and technology, 31(18), 1996, pp. 2455-2471
The demand for stable isotopes in physical and chemical research and i
n medical diagnostics is growing, and the gas centrifuge process is ab
le to provide large quantities of stable isotopes. A set of diffusion
equations describing separation in a gas centrifuge for a multicompone
nt mixture is established. These equations involve general diffusion c
oefficients. Using the radial averaging method and the simplified diff
usion transport vector for a multicomponent isotopic mixture, nonlinea
r partial differential equations are transformed to a set of nonlinear
ordinary differential equations. An iteration method for the solution
is presented. The relationship between the separation factor and the
mass difference, gamma(ij) = gamma(O)(Mj-Mi), is shown to be in agreem
ent with both the computational and the experimental results with very
high precision.