SOLUTION OF THE DIFFUSION-EQUATIONS IN A GAS CENTRIFUGE FOR SEPARATION OF MULTICOMPONENT MIXTURES

Citation
Ct. Ying et al., SOLUTION OF THE DIFFUSION-EQUATIONS IN A GAS CENTRIFUGE FOR SEPARATION OF MULTICOMPONENT MIXTURES, Separation science and technology, 31(18), 1996, pp. 2455-2471
Citations number
19
Categorie Soggetti
Engineering, Chemical",Chemistry
ISSN journal
01496395
Volume
31
Issue
18
Year of publication
1996
Pages
2455 - 2471
Database
ISI
SICI code
0149-6395(1996)31:18<2455:SOTDIA>2.0.ZU;2-A
Abstract
The demand for stable isotopes in physical and chemical research and i n medical diagnostics is growing, and the gas centrifuge process is ab le to provide large quantities of stable isotopes. A set of diffusion equations describing separation in a gas centrifuge for a multicompone nt mixture is established. These equations involve general diffusion c oefficients. Using the radial averaging method and the simplified diff usion transport vector for a multicomponent isotopic mixture, nonlinea r partial differential equations are transformed to a set of nonlinear ordinary differential equations. An iteration method for the solution is presented. The relationship between the separation factor and the mass difference, gamma(ij) = gamma(O)(Mj-Mi), is shown to be in agreem ent with both the computational and the experimental results with very high precision.