T. Sasaki et al., INTERPLAY OF THE SPIN-DENSITY-WAVE STATE AND MAGNETIC-FIELD IN THE ORGANIC CONDUCTOR ALPHA-(BEDT-TTF)(2)KHG(SCN)(4), Physical review. B, Condensed matter, 54(18), 1996, pp. 12969-12978
Magnetic phase diagram of a quasi-two-dimensional organic conductor al
pha-(BEDT-TTF)(2)KHg(SCN)(4) is revisited from a viewpoint of magnetic
torque measurements in high fields up to 30 T. A phase boundary that
is interpreted as a metal-spin density wave (SDW) phase transition is
found by using torque measurements. It is shown that this phase bounda
ry is clearly distinguished from so-called kink transition of the magn
etoresistance. We demonstrate that the transition temperature defined
by the midpoint of the broad phase transition is almost independent on
magnetic field up to 23 T. Onset temperature of the transition shifts
from about 8 K at H = 0 T to higher temperatures with increasing of a
magnetic field, and tends to be saturated. The onset line of this tra
nsition follows well the theoretical expectation that SDW has to be st
abilized by a magnetic field. This allows us to estimate such importan
t band parameters of the quasi-one-dimensional section of the Fermi su
rface as an effective mass, m(1D) similar or equal to (0.5 +/- 0.1)m(0
), and an upper limit of an imperfect nesting bandwidth t(c)(') simila
r or equal to (10 +/- 1) K. The other phase boundaries determined by t
he position of the kink and hysteresis properties of the magnetoresist
ance are interpreted as subphases inside the SDW phase. Inside the SDW
phase, we find an additional phase boundary at the temperature-indepe
ndent field of 23 T, which corresponds to the appearance of de Haas-va
n Alphen oscillations on a magnetic torque curve. At the 23 T boundary
, both the effective mass m, and the Dingle temperature, T-D, change
their values from m = (1.67 +/- 0.05) m(0) and T-D = 3.7 - 4.0 K in l
ow magnetic field region to (1.95 +/- 0.05) m(0) and 2.5 - 2.8 K in hi
gh field region. The latter phenomenon is discussed in terms of a reco
nstruction of the Fermi surface due to the SDW formation. Hysteresis o
f the magnetoresistance observed in one of the subphases inside the SD
W phase is studied in detail by measuring both the temperature and the
magnetic field dependences.