A Michelson interferometer was used to study the quadratic electro-opt
ic effect in KDP. The values for three individual coefficients, determ
ined for the first time by interferometric means, are g(1111) = -4.0,
g(3311) = -0.6, and g(2211) = 0.2 (in units of 10(-20) m(2) V-2). The
lattice contribution, which forms the dominant part of g(1111) and g(3
311), is discussed in terms of the bond polarizability model. The resu
lts provide further evidence that the third-order bond polarizability
is of comparable magnitude for crystals of different structure and com
position.