Fe films ranging in thickness from 6 to 90 Angstrom have been prepared
on Ni layers with constant thickness of 140 Angstrom grown on Si(100)
in ultrahigh vacuum. Magnetic properties have been studied by spin-po
larized neutron reflection and superconducting quantum interference de
vice magnetometry and structural properties have been investigated by
small-angle x-ray reflectometry and reflection high-enegy electron dif
fraction. As the main result of this work it is shown that the magneti
c states of the Fe films strongly depend on their thicknesses. For Fe
layers less than or equal to 32 Angstrom, the average magnetic Fe mome
nts come out to be very low around 0.2 mu(B). For Fe layers greater th
an or equal to 60 Angstrom, the Fe moments increase by a factor of abo
ut 10 close to the value known for bulk iron. Most probably these chan
ges can be attributed to a structural phase transition of the Fe films
from fee-like to bce with increasing Fe layer thickness. Fe films bel
ow 32 Angstrom are either antiferromagnetic or exhibit almost vanishin
g Fe moments. The discussion includes a comparison of our results for
Fe/Ni bilayers with results published for Fe/Ni multilayers and for Fe
films on Cu.