During the last three decades the experimental manipulations of whole
ecosystems have been shown to be a useful and widely used tool for inv
estigation of the effects of air pollution, air pollution reduction st
rategies and management practices on the health and productivity of fo
rests and the acidification of catchments and fresh waters. Generally
the aims have been to investigate the impact of a continued or increas
ed load of air pollutants on the ecosystems, and the possibilities of
reversing the acidifying effects by soil amelioration, addition of buf
fer acting substances or by removal of the air pollutants. Along with
the field experiments, models have been developed to predict future ef
fects and dynamics in the ecosystems under different air pollution sce
narios. The present paper gives an overview of experimental field mani
pulation studies and examples of results obtained with the acidificati
on model MAGIC. All the acidification recovery studies performed so fa
r have shown that a reduced input of S to the ecosystem immediately fr
om the first year resulted in reduced output, although the expected pa
rallel reduction in output of Al and H+ did not occur until some years
later, or not at all. The MAGIC model generally predicts the results
of both acidification and timing field experiments very well, apart fr
om minor discrepancies in year-to-year variability around the observed
trends. Several experimental studies have confirmed that reduced inpu
t of acidity or increased input of base cations caused no or only slig
ht changes in the pH in the soil. The buffer processes of the soil may
cause the effects to be restricted to the very top soil layer, unless
the manipulations were very strong. It is concluded that experimental
field studies have increased our understanding of the complexity of t
he ecosystem and highlighted the need for studies integrating field an
d laboratory work.