MANY-BODY EFFECTS IN THE STATIC STRUCTURE OF DENSE KRYPTON AND XENON

Citation
J. Youden et Pa. Egelstaff, MANY-BODY EFFECTS IN THE STATIC STRUCTURE OF DENSE KRYPTON AND XENON, Physics and chemistry of liquids, 28(2), 1994, pp. 79-94
Citations number
36
Categorie Soggetti
Chemistry Physical","Physics, Condensed Matter
ISSN journal
00319104
Volume
28
Issue
2
Year of publication
1994
Pages
79 - 94
Database
ISI
SICI code
0031-9104(1994)28:2<79:MEITSS>2.0.ZU;2-D
Abstract
The effects of many-body interactions in the static structure of dense gaseous krypton (for 0.9-2.1 rho(c), where rho(c) is the critical den sity) and xenon (for 2.2-2.6 rho(c)) were investigated in the momentum transfer range 4 less than or equal to Q less than or equal to 42 nm( -1), through comparisons of the measured structure factors S(Q) with t hose calculated through the MHNC-CRS integral equation by Reatto and T au. One property investigated is the small increase in the effective a tomic diameter with increasing density. While the observed variation, as determined through the position of the main diffraction maxima, is similar to that given by the inclusion of the Axilrod-Teller triple-di ploe interaction in the calculation, further small deviations exist wh ich indicate the need for additional many-body terms.