A. Bertelsmann et Rh. Heist, 2-DIMENSIONAL TRANSPORT AND WALL EFFECTS IN THE THERMAL-DIFFUSION CLOUD CHAMBER .1. ANALYSIS AND OPERATIONS CRITERIA, The Journal of chemical physics, 106(2), 1997, pp. 610-623
In this paper we present results of a two-dimensional (z,r) treatment
of the mass and energy transfer processes that occur during the operat
ion of a thermal diffusion cloud chamber. The location of the wall is
considered in solving the mass and energy transport equations, in addi
tion to the vertical distance, z, between the upper and lower plate su
rfaces, We examine the effect of aspect (diameter to height) ratio on
chamber operation; the effects of operation with either a dry or a wet
interior chamber wall on temperature, supersaturation, nucleation rat
e, and total density profiles in the chamber; the effect of overheatin
g the interior of the chamber wall on these conditions within the clou
d chamber; and the effects associated with using different density bac
kground gases on the operation of the chamber. In a second paper, imme
diately following, we apply the formalism and the solutions developed
in this paper to address the important problem of buoyancy-driven conv
ection that can accompany (seemingly normal) operation of thermal diff
usion cloud chambers in nearly all ranges of total pressure and temper
ature. (C) 1997 American Institute of Physics.