Impulsive Stimulated Thermal Scattering (ISTS) is a noninvasive optica
l technique that can be used as a powerful tool for high frequency aco
ustic measurements at solid surfaces. In surface ISTS, two interfering
picosecond laser pulses absorbed at the surface launch counterpropaga
ting surface acoustic waves (SAWs) detected via diffraction of a probe
laser beam. In this paper, we introduce surface ISTS measurements in
the frequency domain using a Fabry-Perot interferometer to analyze the
spectrum of the diffracted light. This spectrally separates the ISTS
signal from light scattered by surface imperfections and enables us to
extend the acoustic frequency range beyond 1 GHz. We demonstrate thic
kness and density determination for a gold film on silica from measure
d SAW velocity dispersion. The results obtained show the potential of
the technique for mechanical characterization of him as thin as 0.1 mu
m or less.