Ce3+:LuLiF4 is shown to have a broad gain spectrum, which is attractiv
e for short-pulse applications. A large small-signal gain over 6 dB/cm
and a sufficiently large saturation fluence of 50 mJ/cm(2) were obser
ved for 10-ns probe pulses under KrF excimer laser pumping. In a confo
cal four-pass configuration, 17-dB amplification was demonstrated for
325-nm picosecond pulses, and 20-dB gain was demonstrated for cw laser
light.