We present a novel method for three-dimensional optical data storage t
hat has submicrometer size resolution, provides a large contrast in in
dex of refraction, and is applicable to a wide range of transparent ma
terials. Bits are recorded by use of a 0.65-N.A objective to focus 100
-fs laser pulses inside the material. The laser pulse produces a submi
crometer-diameter structurally altered region with high contrast in in
dex of refraction. We record binary information by writing such bits i
n multiple planes and read it out with a microscope objective with a s
hort depth of field. We demonstrate data storage and retrieval with 2-
mu m in-plane bit spacing and 15-mu m interplane spacing (17 Gbits/cm(
3)). Scanning electron microscopy and atomic force microscopy show str
uctural changes confined to an area 200 nn in diameter. (C) 1996 Optic
al Society of America.