Laser generation with modified poly(methyl methacrylate) (MPMMA)-doped
matrices with several different types of Rhodamine-based dyes was obt
ained. Pumping with a frequency-doubled and-switched Nd:YAG laser was
used. During the experiments, high conversion efficiency was achieved.
The strong nonlinear dependence of the operating lifetime and the con
version efficiency of material tested on the pump-pulse-repetition rat
e was observed. Possible mechanisms responsible for the conversion-eff
iciency drop and the useful lifetime of the material are discussed.