ABATEMENT OF N2O EMISSIONS FROM CIRCULATING FLUIDIZED-BED COMBUSTION THROUGH AFTERBURNING

Citation
L. Gustavsson et B. Leckner, ABATEMENT OF N2O EMISSIONS FROM CIRCULATING FLUIDIZED-BED COMBUSTION THROUGH AFTERBURNING, Industrial & engineering chemistry research, 34(4), 1995, pp. 1419-1427
Citations number
11
Categorie Soggetti
Engineering, Chemical
ISSN journal
08885885
Volume
34
Issue
4
Year of publication
1995
Pages
1419 - 1427
Database
ISI
SICI code
0888-5885(1995)34:4<1419:AONEFC>2.0.ZU;2-G
Abstract
A method for the abatement of N2O emission from fluidized bed combusti on has been investigated. The method consists of burning a secondary f uel after the normal circulating fluidized bed combustor. Liquefied pe troleum gas (LPG), fuel oil, pulverized coal, and wood, as well as saw dust, were used as the secondary fuel. Experiments showed that the N2O emission can be reduced by 90% or more by this technique. The resulti ng N2O emission was principally a function of the gas temperature achi eved in the afterburner and independent of afterburning fuel, but the amount of air in the combustion gases from the primary combustion also influences the results. No negative effects on sulfur capture or on N O or CO emissions were recorded. In the experiments, the primary cyclo ne of the fluidized bed boiler was used for afterburning. If afterburn ing is implemented in a plant optimized for this purpose, an amount of secondary fuel corresponding to 10% of the total energy input should remove practically all N2O. During the present experiments the seconda ry fuel consumption was greater than 10% of the total energy input due to various losses.