MODEL CALCULATION OF THE OPTICAL SUSCEPTI BILITIES TAKING ACCOUNT OF THE SPATIAL-DISPERSION OF NONLINEARITY IN NONLINEAR SPECTROSCOPY OF SOLUTIONS OF CHIRAL MOLECULES

Authors
VOLKOV SN KONOVALOV NI KOROTEEV NI MAKAROV VA
Citation
Sn. Volkov et al., MODEL CALCULATION OF THE OPTICAL SUSCEPTI BILITIES TAKING ACCOUNT OF THE SPATIAL-DISPERSION OF NONLINEARITY IN NONLINEAR SPECTROSCOPY OF SOLUTIONS OF CHIRAL MOLECULES, Kvantovaa elektronika, 22(1), 1995, pp. 71-74
Citations number
8
Categorie Soggetti
Physics, Applied","Engineering, Eletrical & Electronic
Journal title
Kvantovaa elektronika → ACNP
ISSN journal
03687147
Volume
22
Issue
1
Year of publication
1995
Pages
71 - 74
Database
ISI
SICI code
0368-7147(1995)22:1<71:MCOTOS>2.0.ZU;2-F
Abstract
A semiclassical oscillator model, proposed for the interaction of ligh t with complex chiral molecules, takes account of the spatial dispersi on of the susceptibility nonlinearity. The components of the macroscop ic tensors of the nonlinear optical susceptibilities of the second, th ird, and fourth order are calculated for an isotropic gyrotropic mediu m. The calculation is accurate up to terms which are linear in respect of the spatial dispersion parameter and which describe respectively t he sum-frequency generation, CARS (omega(a) = 2 omega-omega(1)), and t he process omega(b) = 3 omega-omega(1).