B. Scholten et al., EXCITATION-FUNCTIONS OF TE-124(P,XN)I-124,I-123 REACTIONS FROM 6MEV TO 31MEV WITH SPECIAL REFERENCE TO THE PRODUCTION OF I-124 AT A SMALL CYCLOTRON, Applied radiation and isotopes, 46(4), 1995, pp. 255-259
Citations number
29
Categorie Soggetti
Nuclear Sciences & Tecnology","Radiology,Nuclear Medicine & Medical Imaging
Excitation functions were measured by the stacked-foil technique for (
p, xn) reactions on highly enriched Te-124 in the proton energy range
of 6-31 MeV. Thin uniform films of Te-124 on Ti-backing were prepared
by an electrodeposition method. Above 17 MeV our data agree within exp
erimental errors with the literature values, thus validating the I-123
-yields and I-124-impurity levels associated with the Te-124(p, 2n)I-1
23 production process. Detailed measurements near the threshold of the
Te-124(p, n)I-124 reaction, on the other hand, show that, contrary to
the general assumption, the thick target yield of I-124 is fairly hig
h, amounting to 20 MBq (0.54 mCi)/mu Ah over the optimum energy range
E(p) = 13 --> 9 MeV. A comparison of the three suggested routes for th
e production of I-124, viz. Te-124(d, 2n)-, Te-126(p, 3n)-, and Te-124
(p, n)-processes, is given. The yield and impurity-level data suggest
that the Te-124(p, n)I-124 reaction has a great potential for producti
on at a small cyclotron.