A study is presented of endohedral muonium (Mu = mu(+)e(-)) in a funct
ionalized fulleroid, the 6, 5 isomer of C61H2. The temperature indepen
dence of the muonium depolarization rate implies that in the timescale
of the mu SR experiment no isotropic reorientation regime sets in eve
n at 280 K. The depolarization appears dominated by the interaction of
Mu with methylene protons. No anisotropy of the hyperfine interaction
was directly detected within experimental accuracy; an upper limit fo
r the anisotropy can be fixed to 600 kHz by a transverse field measure
ment.