Pulsed laser deposition (PLD) of niobium telluride was performed by va
porisation of NbTe2 bulk targets with subsequent deposition of the abl
ation plume on heated silicon substrates. The laser energy density ont
o the target and the temperature of the substrate appear to play a maj
or role in the quality of the deposited films. Correlations between th
ese two parameters and the film composition on the one hand, and the s
tructural properties on the other, were sought by systematic elemental
and X-ray diffraction analysis. The deposition conditions for well-cr
ystallized PLD films belonging to the Nb5Te4 (1D) structural type with
strong (110) preferential orientation were demonstrated for the first
time.