M. Corti et al., LA-139 NQR RELAXATION AND MU-SR STUDY OF LA2CU1-XZNXO4, Nuovo cimento della Societa italiana di fisica. D, Condensed matter,atomic, molecular and chemical physics, biophysics, 16(10-11), 1994, pp. 1793-1797
La-139 NQR spectra, mu SR precessional frequencies and NQR relaxation
rates W driven by the Cu2+ spin fluctuations are used to study the sta
tic magnetic properties and the low-energy spin excitations upon subst
itution of Zn2+ (S=0) for Cu2+ (S=1/2) in the antiferromagnetic (AF) p
hases of La2Cu1-xZnxO4. It is found that the Neel temperatures T-N dec
rease with IL almost linearly, with initial suppression rate close to
4, while the sublattice magnetization is only slightly affected, close
to the behaviour expected for a 2D S=1/2 Heisenberg AF in the framewo
rk of dilution model. Also the spin wave spectrum appears slightly aff
ected by Zn doping, with moderate effects possibly related to disorder
in the AF interactions and/or to finite size. A novel and remarkable
effect is observed for T less than or equal to 100 K. The relaxation r
ates W show large maxima, with x-dependent W-max and T-max. This pheno
menon is attributed to the cooperative freezing of local magnetic mome
nts induced by Zn on Cu orbitals. Information on the characteristic fl
uctuation frequencies and on the spin-glass state superimposed to the
AF matrix are thus obtained.