V. Chernyak et S. Mukamel, LEVEL CORRELATIONS AND DEPHASING-INDUCED RESONANCES IN MOLECULAR AGGREGATES, Physica status solidi. b, Basic research, 189(1), 1995, pp. 67-73
Dephasing-induced resonances in the nonlinear optical response of mole
cular aggregates are expressed in terms or level correlations. The thi
rd-order optical response is related to the three-dimensional spectral
density function chi(epsilon', epsilon,epsilon E''), Expressions for
chi(epsilon', epsilon, epsilon'') derived using the Frenkel exciton mo
del show the existence of collective (dephasing-induced) resonances.