LEVEL CORRELATIONS AND DEPHASING-INDUCED RESONANCES IN MOLECULAR AGGREGATES

Citation
V. Chernyak et S. Mukamel, LEVEL CORRELATIONS AND DEPHASING-INDUCED RESONANCES IN MOLECULAR AGGREGATES, Physica status solidi. b, Basic research, 189(1), 1995, pp. 67-73
Citations number
12
Categorie Soggetti
Physics, Condensed Matter
ISSN journal
03701972
Volume
189
Issue
1
Year of publication
1995
Pages
67 - 73
Database
ISI
SICI code
0370-1972(1995)189:1<67:LCADRI>2.0.ZU;2-1
Abstract
Dephasing-induced resonances in the nonlinear optical response of mole cular aggregates are expressed in terms or level correlations. The thi rd-order optical response is related to the three-dimensional spectral density function chi(epsilon', epsilon,epsilon E''), Expressions for chi(epsilon', epsilon, epsilon'') derived using the Frenkel exciton mo del show the existence of collective (dephasing-induced) resonances.