ORDERING DUE TO DISORDER IN AN ANTIFERROMAGNET WITH CONTINUOUSLY DEGENERATE NEEL GROUND-STATE - A COMBINED NEUTRON-DIFFRACTION AND MAGNETIZATION STUDY OF (FEXGA1-X)(2) CA3GE3O(12)
T. Bruckel et al., ORDERING DUE TO DISORDER IN AN ANTIFERROMAGNET WITH CONTINUOUSLY DEGENERATE NEEL GROUND-STATE - A COMBINED NEUTRON-DIFFRACTION AND MAGNETIZATION STUDY OF (FEXGA1-X)(2) CA3GE3O(12), Zeitschrift fur Physik. B, Condensed matter, 97(3), 1995, pp. 391-401
In general, fluctuations suppress order in ''conventional'' many body
systems. Here we present results of an experimental study intended to
test recent ideas about how quantum, thermal and quenched noise may in
duce ordering in highly frustrated magnets. Our model system, the garn
et Fe2Ca3Ge3O12, is an antiferromagnet with a continuously degenerate
Neel ground state. We report combined magnetization- and neutron diffr
action studies on the dilution series (FexGa1-x)(2)Ca3Ge3O12 (0 less t
han or equal to x less than or equal to 1). We propose a complex magne
tic phase diagram with a spin glass phase around x = 0.5. Within a wid
e concentration range, we observe a micro-domain state, where true lon
g range order is never established. The correlation lengths lie betwee
n some 300 Angstrom for x = 0.4 and greater than or equal to 900 Angst
rom for x greater than or equal to 0.8. We relate our findings to rece
nt theories about how fluctuations select a definite spin structure in
highly frustrated antiferromagnets. This leads us to propose two diff
erent spin structures for the pure and the diluted samples: our observ
ations are in accordance with a stabilization of a collinear structure
via quantum and thermal fluctuations, while quenched stoichiometric d
isorder lifts the ground state degeneracy but favours a canted spin ar
rangement.