The surface tension of copper-nickel alloys was measured, both as func
tions of concentration and temperature, using electromagnetic levitati
on and the oscillating drop technique. The measurements covered the en
tire concentration range from c(Cu) = 0 to 100%, and a temperature ran
ge that included the molten as well as the undercooled regime. The res
ults agree well with a model based on Butler's formula for the surface
tension and chemical potentials measured in the bulk liquid phase. Th
is allows one to calculate the surface segregation of this system.