Jm. Auerhammer et al., EFFICIENT FREQUENCY-DOUBLING OF PS-PULSES FROM A FREE-ELECTRON LASER IN ZNGEP2, Optics communications, 118(1-2), 1995, pp. 85-89
We report second-harmonic generation in ZnGeP2 in the mid-IR using a h
igh power, short pulse, free-electron laser. For fundamental wavelengt
hs between 5.5 to 9.0 mu m external efficiencies for second-harmonic g
eneration up to 49% have been reached, which is close to the theoretic
al limit. At longer wavelengths the efficiency is reduced as a result
of absorption in the crystal.