The multiple scattering background in Compton scatter imaging at 662 k
eV is studied, both experimentally and by Monte Carlo radiation transp
ort calculations, as a function of the scattering angle, scattering ma
terial (aluminium, brass and tin) and object thickness. A double-peak
structure was observed in the pulse-height distribution for the thicke
r brass and tin objects and at the larger scattering angles (90 degree
s and 120 degrees). In addition to the Compton peak, a second peak app
eared at a higher energy. Monte Carlo transport simulations have revea
led the origin of the second peak: photons that have scattered exactly
twice before reaching the detector. The ratio of the multiple-scatter
ed radiation to the total radiation detected was calculated as a funct
ion of the energy-window width around the Compton peak and scattering
angle. The results of this study may help in the design of future Comp
ton scatter imaging apparatus.