INTERACTING TUNNELING STATES - A HOLE-BURNING STUDY OF SPECTRAL DIFFUSION

Citation
G. Hannig et al., INTERACTING TUNNELING STATES - A HOLE-BURNING STUDY OF SPECTRAL DIFFUSION, Molecular crystals and liquid crystals science and technology. Section A, Molecular crystals and liquid crystals, 291, 1996, pp. 11-16
Citations number
13
Categorie Soggetti
Crystallography
ISSN journal
1058725X
Volume
291
Year of publication
1996
Pages
11 - 16
Database
ISI
SICI code
1058-725X(1996)291:<11:ITS-AH>2.0.ZU;2-M
Abstract
Performing long-time thermal equilibrium measurements of spectral diff usion broadening of photochemical holes, we recently established an al gebraic time dependence of the dynamics of two-level system (TLS), whi ch we interpret in terms of TLS-TLS coupling (Phys. Rev. Lett. 76 (199 6) 2085). For this purpose we utilized the continuous cooling property of our He-3/He-4 cryostat. To extend the accessible temperature range we have constructed a cryostat which allows optical experiments lasti ng several weeks at temperatures of 1.5K and above. Here we report dat a obtained at 2.0K in a time range from 10 s to 10(6) s. Interpreted i n the framework mentioned above, the results indicate the onset of a t hermally induced break-up of the TLS-TLS coupling.