G. Witte et al., HELIUM-ATOM-SCATTERING STUDY OF THE DISPERSION-CURVES OF STEP-LOCALIZED PHONONS ON CU(211) AND CU(511), Physical review. B, Condensed matter, 52(3), 1995, pp. 2165-2176
The surface phonon dispersion curves of two different regularly steppe
d vicinal copper surfaces have been measured using high resolution ine
lastic helium-atom scattering. The Cu(211) and Cu(511) surfaces were c
hosen since they have comparable step distances but different terrace
orientations (111) and (100), respectively. The Rayleigh mode was meas
ured over the entire Brillouin zone along azimuths parallel and perpen
dicular to the step edge directions. For both surfaces backfolding of
the Rayleigh mode was observed along the direction perpendicular to th
e step edges, while parallel to the step edges, a step localized mode
with optical character and a weak dispersion were also found. For the
Cu(511) surface, an additional longitudinal mode and an energy gap for
the Rayleigh mode at the zone boundary could be identifed, whereas on
Cu(211), an additional horizontal mode could be identified. The low z
one boundary energy observed for the latter mode can be related to the
relaxation of the step atoms. The experimental data can be well expla
ined by theoretical slab calculations in the framework of a single for
ce constant model.