P. Kurpick et al., RELATIVISTIC AB-INITIO INTERPRETATION OF L-K VACANCY SHARING IN ION-SOLID-TARGET COLLISIONS, Physical review. A, 52(3), 1995, pp. 2132-2135
The first experiments measuring the impact-parameter-dependent L-K vac
ancy sharing in ion-solid-target collisions started almost two decades
ago. A rather qualitative explanation of the vacancy sharing process
was achieved in the framework of the 2p pi-2p sigma coupling scheme de
veloped by Briggs and Taulbjerg, but for most of the collision systems
significant discrepancies remained. Even a multiple collision calcula
tion using the 2p pi-2p sigma coupling scheme, as undertaken by Schuch
et al., did not improve the agreement with the experimental results a
nd left a lack of an explanation, calling for first-principles calcula
tions. Using our ab initio relativistic Dirac-Fock-Slater many-electro
n basis set method, we confirm that both a qualitative and quantitativ
e explanation can be given for the L-K vacancy sharing process in heav
y ion-solid-target collisions. As an example, we compare our results w
ith measurements for 108-MeV Br on Ni-solid targets.