Two new anthrones were isolated from Harungana madagascariensis in add
ition to a known anthrone, two xanthones, four anthraquinones and two
flavonoids. The structures of the two anthrones were determined to be
1,3,8-trihydroxy-4,5-diisoprenyl-7-methylanthrone (harunganol A) and 1
,3,8-trihydroxy-4,5,7-triisoprenyl-7-methyl- anthrone (harunganol B) b
y spectroscopic analysis. The other anthrone, 8-dihydroxy-2-isoprenyl-
3-methoxy-6-methylanthrone which has been once derived from natural pr
oduct, and one xanthone, 1,5,6-trihydroxy-7-methoxyxanthone which has
been synthesized earlier were isolated for the first time as genuine n
atural products.