Single-crystal films of permalloy (Ni80F20) were grown on Cu(001) seed
layers oriented epitaxially with Si(001). The microstructural propert
ies were measured using in-situ reflection high-energy electron diffra
ction, and ex-situ transmission electron microscopy, x-ray diffraction
, and atomic force microscopy, whereas the magnetic properties were pr
obed using in-situ magneto-optic Kerr effect and ex-situ vibrating sam
ple magnetometry. Anisotropic magnetoresistance and resistivity for so
me of the samples were also measured. The coercivity for thinner (less
than or equal to 5 nm) Ni80Fe20 was significantly higher (10-20 Oerst
eds) than polycrystalline films deposited on SiO2/Si, and was also hig
her than films deposited on lattice-matched CuxNi1-x alloys. These mag
netic properties were explained using a theoretical model involving in
teraction of domain walls with defects such as misfit dislocations and
coherent islands, due to the mismatch between Ni80Fe20 and Cu.