As. Choe et al., EFFECTS OF A LASER-PULSE PHOTOIONIZING AN EFFECTIVELY EXCITED 3-LEVELATOM ON THE ION YIELD, Journal of physics. B, Atomic molecular and optical physics, 28(17), 1995, pp. 3821-3829
The population inversion in a three-level atomic system, interacting w
ith two coherent laser pulses, occurs from the first level to the thir
d level at the optimal detunings of the laser frequencies near the two
-photon resonance. An examination is performed to see whether the ener
gy density and time-delay of the photoionizing laser can significantly
influence the ion yield for the case where the atom interacts with tw
o coherent pulses and one photoionizing pulse incoherently coupled. Th
e well-known three-colour, three-step, three-photon ionization scheme,
which is available for the selective photoionization of Yb-168, is ch
osen for use in this research with the Bloch equation. It is revealed
that the proper time-delay and energy density enable us to achieve hig
her efficiency for the selective photoionization of Yb-168, regardless
of the Doppler-broadening, though the efficiency and selectivity of c
oherent excitation are prominently enhanced by applying the optimal de
tunings.