Jg. Mihaychuk et al., TIME-DEPENDENT 2ND-HARMONIC GENERATION FROM THE SI-SIO2 INTERFACE INDUCED BY CHARGE-TRANSFER, Optics letters, 20(20), 1995, pp. 2063-2065
We have observed that the second-harmonic signal generated from oxidiz
ed Si(001) varies on a time scale of several seconds in experiments in
volving a fundamental beam of lambda = 770 nm, 110-fs pulses at 76 MHz
. We suggest that the temporal behavior arises from absorption of weak
(< 100-fW average power) third-harmonic light generated in air or in
the sample, inducing charge transfer across the Si-SiO2 interface and
trapping in the oxide layer. Detrapping has been determined to take se
veral minutes. (C) 1995 Optical Society of America