L. Paschedag et al., HIGH-FREQUENCY ELECTRON-NUCLEAR DOUBLE-RESONANCE AT 239 GHZ USING A FAR-INFRARED LASER SOURCE, Review of scientific instruments, 66(10), 1995, pp. 5098-5099
We report on the application of N-14 electron nuclear double resonance
(ENDOR) at 8.5 T and 239 GHz (lambda=1.2 mm) in a gamma-irradiated be
taine arsenate single crystal. A laser was used as a far-infrared radi
ation source in a transmission-type electron paramagnetic resonance (E
PR) setup without a cavity. The four expected nitrogen ENDOR lines wer
e observed, but due to insufficient saturation of the EPR transitions
the signal/noise ratio was not larger than 10 and the signals vanished
at temperatures above 20 K. (C) 1995 American Institute of Physics.