Ya. Shukolyukov et Ap. Meshik, CHEMICALLY FRACTIONATED URANIUM FISSION X ENON IN MANTLE ROCKS, GASESAND TERRESTRIAL ATMOSPHERE, Geohimia, (8), 1995, pp. 1072-1093
A new conception on the origin of isotopic composition of terrestrial
atmospheric xenon has been suggested, According this conception the ex
cess of Xe-129 originates from I-129 that is a product of neutron indu
ced fission of U-235, but not from primordial I-129 trapped by the Ear
th during its accretion. Having analyzed all published data on xenon i
sopotic composition mantle rocks and gases, the obvious correlation be
tween excess Xe-129 and excesses in other xenon isotopes, particularly
in Xe-132 and Xe-131, has been found. The isotopic pattern of excess
xenon corresponds to that of CFF-Xe, the latter being the result of ch
emical fractionation of radioactive Xe precursors in beta-chains deriv
ed from the fission of heavy nuclei. The experimental study of xenon r
eleased from the materials of naturally occurring nuclear reactor in O
klo, of Colorado type uranium deposits and of some other objects prove
s that the generation of chemically fractionated fission xenon under n
atural conditions is quite possible. The presence of CFF-Xe in terrest
rial atmosphere removes difficulties in the interpretation of present
isotopic abundances of atmospheric xenon: neither hypothetical U-Xe, n
or searching of exotic mechanism of selective isotopic fractionation o
f AVCC-Xe are needed any more. The performed balance calculation showe
d that the generation of required amount of CFF-Xe was possible in the
course of neutron induced fission of U-235 migrating into the core du
ring the Earth's differentiation. In the context of proposed conceptio
n those models of the Earth's degassing that based upon the origin of
Xe-129 from primordial I-129 become questionable.