We have grown MnBi1-xSbx alloy films on mica and glass substrates unde
r UHV conditions, and performed a systematic study of the structural,
magnetic and magneto-optic properties on films in the concentration ra
nge 0 less than or equal to x less than or equal to 0.4. Sharp Reflect
ion High Energy Electron Diffraction (RHEED) patterns were observed fo
r samples grown on mica substrates, indicating epitaxial growth. X-ray
diffraction patterns of MnBi1-xSbx grown on glass substrates show the
se films to be highly textured, with the c-axis parallel to the substr
ate normal. We found that only samples with Mn concentration above 50
at. % exhibited good magneto-optical properties. Perpendicular magneti
zation and Kerr rotation larger than 0.5 degrees were observed for sam
ples with Sb concentration less than 8 at. % in mica and 4 at. % on gl
ass. For larger concentrations of Sb, the coercivity increased rapidly
while Kerr rotation decreased. Samples grown on both types of substra
tes showed an increase in the Kerr rotation and ellipticity with decre
asing light wavelengths. The off-diagonal E-field reflectivity, r(xy),
which describes the magneto-optic efficiency of the sample, is larger
than that reported for TbFeCo layers.