Infrared and Raman analyses on the configuration of hydrogenated amorp
hous carbon (a-C:H) thin films on monocrystalline Ge and Si substrates
have been carried out. Models of the short range order and of the non
-equilibrium crystallization aggregation of the films are proposed bas
ed on the analysis results and previous works by Smith [1, 2], Lu and
Wang [3] and Witten and Sander [4]. The computer simulated aggregates,
according to the models, are fractals with the dimension 1.81 +/- 0.0
6. The films have been crystallized by laser illustration quenching. T
he fractal dimension of the experimentally obtained aggregates is in a
greement with the simulation result.