The second-harmonic generation with evanescent wave technique was used
to measure the efficiency of second-harmonic generation of an organic
colored powder that absorbs the second-harmonic wave, and it was comp
ared to the electro-optic coefficient. The refractive index of the sam
ple at the second-harmonic frequency is complex. The effective refract
ive index was obtained by measuring reflectivity at the interface betw
een the sample and the prism. This technique is potentially useful for
surveying electro-optic materials.