J. Mathon et al., THEORY OF THE SYSTEMATIC VARIATION OF THE EXCHANGE COUPLING STRENGTH IN MAGNETIC MULTILAYERS, Journal of magnetism and magnetic materials, 127(3), 1993, pp. 120000261-120000266
The amplitude of the exchange coupling between Co or Fe layers separat
ed by different nonmagnetic transition metal spacers is observed to de
crease exponentially with decreasing number of electrons per atom in t
he spacer. An earlier theory based on size quantization of magnetic ca
rriers in the spacer layer is generalized to show that the systematic
variation of the coupling strength across the transition metal series
is due to a misalignment between the ferromagnet and spacer bands whic
h increases with increasing number of holes in the spacer. A general p
hysical picture of the effect based on conservation laws and phase spa
ce availability is presented. Tight-binding calculations confirm the v
alidity of the band misalignment theory. It is also shown that the sys
tematic variation of the coupling strength cannot be explained by simp
le RKKY type theories.