STRONG BULK MAGNETIC DIPOLE INDUCED SECOND-HARMONIC GENERATION FROM C-60

Authors
KOOPMANS B JANNER AM JONKMAN HT SAWATZKY GA VANDERWOUDE F
Citation
B. Koopmans et al., STRONG BULK MAGNETIC DIPOLE INDUCED SECOND-HARMONIC GENERATION FROM C-60, Physical review letters, 71(21), 1993, pp. 3569-3572
Citations number
16
Categorie Soggetti
Physics
Journal title
Physical review letters → ACNP
ISSN journal
00319007
Volume
71
Issue
21
Year of publication
1993
Pages
3569 - 3572
Database
ISI
SICI code
0031-9007(1993)71:21<3569:SBMDIS>2.0.ZU;2-I
Abstract
We describe how to separate all surface, interface, and bulk tensor co mponents in optical second-harmonic generation experiments on isotropi c thin films. Using in situ thickness scans and group theoretical argu ments concerning the bulk tensor components, we demonstrate that the s econd-harmonic resonance of C60 at 2HBARomega=3.6 eV is of bulk charac ter, and, quite remarkably, of magnetic dipole induced origin.