The magnetic properties of single-phase 2:17 compounds of the composit
ion Sm2Fe17-xGaxHy were investigated. The substitution of Ga for Fe in
the Sm2Fe17 compound resulted in a substantial increase in the Curie
temperature and, for alloys with x > 2, the formation of a uniaxial ma
gnetic anisotropy at room temperature. The diffusion of hydrogen into
those compounds that exhibit an easy axis anisotropy causes a transiti
on back to a planar anisotropy. This indicates that the presence of in
terstitial hydrogen is detrimental to the hard magnetic properties of
these materials.