One of the principal obstacles to room temperature tensile ductility i
n NiAl is an insufficient number of independent slip systems, due to t
he sole operation of the [100]{011} system. It has been both predicted
and reported that Cr additions to NiAl induce [111]{112} slip, increa
sing the number of independent slip systems to five, a number sufficie
nt for general plasticity. However, no attendant increase in tensile d
uctility has been observed. The present study reexamines the effects o
f Cr on the predominant room temperature slip system in polycrystallin
e NiAl, as a function of Cr content, Ni/Al ratio and processing route.
It is shown that Cr has essentially no effect on the slip system in N
iAl at room temperature, while processing by extrusion, compared with
casting and homogenization, produces a small, yet significant, proport
ion of [110]{110} dislocations. Possible explanations for the discrepa
ncy of the present results with those of previous work are discussed,
as well as the presence and implications of the [110]{110} dislocation
s.