NONLINEAR LASER SPECTROSCOPY OF NONLINEAR SOLVATION

Citation
Bd. Fainberg et al., NONLINEAR LASER SPECTROSCOPY OF NONLINEAR SOLVATION, Journal of nonlinear optical physics and materials, 5(4), 1996, pp. 789-807
Citations number
32
Categorie Soggetti
Physics, Applied",Optics
ISSN journal
02188635
Volume
5
Issue
4
Year of publication
1996
Pages
789 - 807
Database
ISI
SICI code
0218-8635(1996)5:4<789:NLSONS>2.0.ZU;2-Y
Abstract
In this study we show that the transient four-photon spectroscopy with pulses longer than the electronic transition dephasing can be used fo r nonlinear solvation study, i.e., when the linear response for the so lvation dynamics breaks down. We have obtained new formulae describing the time evolution of the moments of the nonlinear optical spectra an d, in particular, the time resolved fluorescence in the case of nonlin ear solvation.