Ec. Cheung et al., MEASUREMENTS OF 2ND-ORDER NONLINEAR-OPTICAL COEFFICIENTS FROM THE SPECTRAL BRIGHTNESS OF PARAMETRIC FLUORESCENCE, Optics letters, 19(3), 1994, pp. 168-170
We report a new technique for determining second-order nonlinear optic
al coefficients that uses the spectral brightness of spontaneous param
etric fluorescence. Measurements with this technique on two separate A
gGaS2 crystals yielded values of 22.9 and 24.3 pm/V for \d36\, and mea
surements on a KTP crystal yielded 4.1 pm/V for \d24\. The uncertainty
of the determined values is approximately +/-10%.