VIBRATIONAL HEATING AND ATOM-TRANSFER WITH THE STM

Citation
Re. Walkup et al., VIBRATIONAL HEATING AND ATOM-TRANSFER WITH THE STM, Journal of electron spectroscopy and related phenomena, 64-5, 1993, pp. 523-532
Citations number
23
Categorie Soggetti
Spectroscopy
ISSN journal
03682048
Volume
64-5
Year of publication
1993
Pages
523 - 532
Database
ISI
SICI code
0368-2048(1993)64-5:<523:VHAAWT>2.0.ZU;2-A
Abstract
The high current density of the STM can result in substantial vibratio nal heating via inelastic electron tunneling. Under certain conditions , the vibrational distribution at a given current-density is approxima tely Maxwell-Boltzmann, with a characteristic temperature that reflect s a balance between excitation by the tunneling electrons and relaxati on processes. A simple expression is given for the steady-state vibrat ional temperature in the presence of tunneling current. Calculations i ndicate that vibrational heating by inelastic tunneling plays an impor tant role in the transfer of Xe atoms between sample and tip surfaces. Directionality of Xe atom-transfer, and applications to other systems are discussed.