Comparisons are drawn between the aerosol cloud microphysical theory i
mplicit in the modeling of Kaufman et al. and the cloud droplet and cl
oud water sulfate concentrations of Leaitch et al. for the purpose of
helping to understand the effect of sulfate particles on climate throu
gh cloud modification. In terms of the range of possibilities and pros
pects for future climate given by Kaufman et al. for the effect of sul
fur on cloud albedo, the data favor the possibility of stronger coolin
g. Scatter in the data makes it impossible to constrain model paramete
rs; however, the comparisons suggest that there may not be a universal
relationship, and that the uncertainties involved in trying to model
this process are large.